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Creators/Authors contains: "Spaepen, Frans"

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  1. ; ; ; ; (, Physical Review E)
    Despite significant advances in particle imaging technologies over the past two decades, few ad- vances have been made in particle tracking, i.e. linking individual particle positions across time series data. The state-of-the-art tracking algorithm is highly effective for systems in which the particles behave mostly independently. However, these algorithms become inaccurate when particle motion is highly correlated, such as in dense or strongly interacting systems. Accurate particle tracking is essential in the study of the physics of dense colloids, such as the study of dislocation formation, nucleation, and shear transformations. Here, we present a new method for particle tracking that incorporates information about the correlated motion of the particles. We demonstrate significant improvement over the state-of-the-art tracking algorithm in simulated data on highly correlated systems." 
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  2. ; ; ; ; ; ; ; ; ; ; et al (, Proceedings of the National Academy of Sciences)
    Significance Self-assembly is one of the central themes in biologically controlled synthesis, and it also plays a pivotal role in fabricating a variety of advanced engineering materials. In particular, evaporation-induced self-assembly of colloidal particles enables versatile fabrication of highly ordered two- or three-dimensional nanostructures for optical, sensing, catalytic, and other applications. While it is well known that this process results in the formation of the face-centered cubic (fcc) lattice with the close-packed {111} plane parallel to the substrate, the crystallographic texture development of colloidal crystals is less understood. In this study, we show that the preferred <110> growth in the fcc colloidal crystals synthesized through evaporation-induced assembly is achieved through a gradual crystallographic rotation facilitated by mechanical stress-induced geometrically necessary dislocations. 
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